分类： 光学 >> 量子光学 提交时间： 2023-02-19
Lufang Liu
Alexey V. Krasavin
Junsheng Zheng
Yuanbiao Tong
Pan Wang
Xiaofei Wu
Bert Hecht
Chenxinyu Pan
Jialin Li
Linjun Li
Xin Guo
Anatoly V. Zayats
Limin Tong
摘要： Nanoparticle-on-mirror plasmonic nanocavities, capable of extreme optical confinement and enhancement, have triggered state-of-the-art progress in nanophotonics and development of applications in enhanced spectroscopies and molecular detection. However, the optical quality factor and thus performance of these nanoconstructs are undermined by the granular polycrystalline metal films used as a mirror. Here, we report an atomically smooth single-crystalline platform for low-loss nanocavities using chemically-synthesized gold microflakes as a mirror. Nanocavities constructed using gold nanorods on such microflakes exhibit a rich structure of plasmonic modes, which are highly sensitive to the thickness of optically-thin (down to ~15 nm) microflakes. The atomically smooth single-crystalline microflakes endow nanocavities with significantly improved quality factor (~2 times) and scattering intensity (~3 times) compared with their counterparts based on deposited films. The developed low-loss nanocavities further allow for the integration with a mature platform of fiber optics, opening opportunities for realizing nanocavity-based miniaturized photonic devices with high performance.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： Random fiber laser (RFL) is a complex physical system that arises from the distributed amplification and the intrinsic stochasticity of the fiber scattering. There has been widespread interest in analyzing the underlying lightwave kinetics at steady state. However, the transient state, such as the RFL build-up and dissipation, is also particularly important for unfolding lightwave interaction process. Here, we investigate for the first time the RFL dynamics at transient state, and track the RFL temporal and spectral evolution theoretically and experimentally. Particularly, with the contribution of randomly distributed feedback, the build-up of RFL shows continuous Verhulst logistic growth curves without cavity-related features, which is significantly different from the step-like growth curve of conventional fiber lasers. Furthermore, the radiation build-up duration is inversely related to the pump power, and the spectral evolution of RFL undergoes two phases from spectral density increase to spectral broadening. From steady-state to pump switch-off state, the RFL output power dissipates immediately, and the remaining Stokes lightwave from the Rayleigh scattering will gradually disappear after one round-trip. This work provides new insights into the transient dynamics features of the RFL.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
Lulu Ye
Weidong Zhang
Aiqin Hu
Hai Lin
Jinglin Tang
Yunkun Wang
Chenxinyu Pan
Pan Wang
Xin Guo
Limin Tong
Yunan Gao
Qihuang Gong
Guowei Lu
摘要： Plasmon decay via the surface or interface is a critical process for practical energy conversion and plasmonic catalysis. However, the relationship between plasmon damping and the coupling between the plasmon and 2D materials is still unclear. The spectral splitting due to plasmon-exciton interaction impedes the conventional single-particle method to evaluate the plasmon damping rate by the spectral linewidth directly. Here, we investigated the interaction between a single gold nanorod (GNR) and 2D materials using the single-particle spectroscopy method assisted with in situ nanomanipulation technique by comparing scattering intensity and linewidth together. Our approach allows us to indisputably identify that the plasmon-exciton coupling in the GNR-WSe2 hybrid would induce plasmon damping. We can also isolate the contribution between the charge transfer channel and resonant energy transfer channel for the plasmon decay in the GNR-graphene hybrid by comparing that with thin hBN layers as an intermediate medium to block the charge transfer. We find out that the contact layer between the GNR and 2D materials contributes most of the interfacial plasmon damping. These findings contribute to a deep understanding of interfacial excitonic effects on the plasmon and 2D materials hybrid.
分类： 光学 >> 量子光学 提交时间： 2023-02-19
摘要： Phonon polaritons in natural anisotropic crystals hold great promise for infrared nano-optics. However, the direct electrical control of these polaritons is difficult, preventing the development of active polaritonic devices. Here we propose the heterostructures of graphene on a biaxial crystal ({\alpha}-phase molybdenum trioxide) slab and theoretically study the hybridized plasmon-phonon polaritons with dependence on the Fermi level of graphene from three aspects: dispersion relationships, iso-frequency contours, and the quantum spin Hall effects. We demonstrate the distinct wavelength tunability of the plasmon-phonon polaritons modes and the optical topologic transitions from open (hyperbolic) to closed (bow-tie-like) iso-frequency contours as the increase of the Fermi level of graphene. Furthermore, we observe the tunable quantum spin Hall effects of the plasmon-phonon polaritons, manifesting propagation direction switching by the Fermi level tuning of the graphene. Our findings open opportunities for novel electrically tunable polaritonic devices and programmable quantum optical networks.
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